• JoomlaWorks Simple Image Rotator
  • JoomlaWorks Simple Image Rotator
  • JoomlaWorks Simple Image Rotator
  • JoomlaWorks Simple Image Rotator
  • JoomlaWorks Simple Image Rotator
  • JoomlaWorks Simple Image Rotator
  • JoomlaWorks Simple Image Rotator
  • JoomlaWorks Simple Image Rotator
  • JoomlaWorks Simple Image Rotator
  • JoomlaWorks Simple Image Rotator
 
  Bookmark and Share
 
 
Master's Dissertation
DOI
https://doi.org/10.11606/D.85.2013.tde-10012014-153128
Document
Author
Full name
Juliana Cristina da Silva
E-mail
Institute/School/College
Knowledge Area
Date of Defense
Published
São Paulo, 2013
Supervisor
Committee
Camargo, Iara Maria Carneiro de (President)
Boscov, Maria Eugenia Gimenez
Figueiredo, Ana Maria Graciano
Title in Portuguese
Mobilidade de As, Cd, Mo, Pb e Zn em colunas de latossolo argiloso com cinza de carvão e contaminação do solo
Keywords in Portuguese
As
cinza de carvão
colunas
metais
solo
Abstract in Portuguese
A contaminação do solo tem sido motivo de preocupação ambiental e de saúde pública, uma vez que o homem depende do seu uso para sobreviver. O resíduo de cinza de carvão, gerado da queima de carvão em usina termoelétrica, é uma das fontes contaminadoras do solo quando disposto de forma inadequada. Os elementos tóxicos da cinza de carvão, quando depositada sobre o solo e exposta à chuva, podem ser lixiviados da cinza para o solo. No solo estes elementos podem ser sorvidos, transportados para a água subterrânea e superficial ou absorvido pelas plantas, o que pode contaminar estas matrizes ambientais. O objetivo do estudo foi avaliar a mobilidade de As, Cd, Mo, Pb e Zn em colunas de Latossolo argiloso com cinza de carvão sobreposta ao solo e avaliar se a retenção destes elementos provoca a contaminação do solo. As colunas foram percoladas com uma solução ácida com pH 4,5 para simular água de chuva, por períodos de 168 e 336 dias. As amostras de cinza de carvão, solo e percolado das colunas foram analisadas quanto à concentração dos elementos e as características físicas, químicas e mineralógicas. O Pb não foi lixiviado da cinza de carvão, portanto, o solo e percolado do solo não foram contaminados por este elemento. Os elementos As, Cd, Mo e Zn foram lixiviados da cinza de carvão e não foram detectados no percolado das colunas, indicando que estes elementos ficaram retidos no solo. A concentração do Mo no solo não foi detectada acima do limite de quantificação do método. A concentração dos elementos foi comparada com os valores orientadores para solos estabelecidos pela CETESB. A maior parte do Zn detectado no solo foi proveniente do próprio solo utilizado no preparo da coluna e a concentração deste elemento no solo foi abaixo do valor de referência (60 mg kg-1). A concentração do Cd no solo foi acima do valor de referência (<0,5 mg kg-1) e abaixo do valor de intervenção (3 mg kg-1). A concentração do As no solo foi acima do valor de intervenção (35 mg kg-1), sendo o único elemento crítico do ponto de vista ambiental.
Title in English
Mobility of As, Cd, Mo, Pb and Zn in clayey oxisol columns with coal fly ash and soil contamination
Keywords in English
As
coal ash
columns
metal
soil
Abstract in English
Soil contamination has been an environmental and public health concern, once the man depends on its use to survive. Coal fly ash generated by coal burning in power plants is one source of soil contamination when it inadequately disposed. Toxic elements from coal fly ash, deposited on soil and exposed to rain, can be leached into the soil. In the soil these elements can be sorbed, transported to groundwater and surface water or even absorbed by plants, which can contaminate these environmental matrices. The aim of study was to evaluate the mobility of As, Cd, Mo, Pb and Zn in clayey oxisol columns with coal fly ash on top soil, and also evaluate if these elements retention leads to soil contamination. The columns were percolated by acidic solution, pH 4.5, to simulate rain water, in periods of 168 and 336 days. The elements concentration and physical, chemical and mineralogical characteristics were determined in coal fly ash, soil and column leachate samples. Lead was not leached from coal fly ash, therefore the soil and the column leachate were not contaminated by this element. The elements As, Cd, Mo and Zn were leached from coal fly ash and were not detected in leachate of soil, that means these elements were retained in soil. The Mo concentration was below the quantification limit of method. The As, Cd and Zn concentrations were compared with the CETESB guideline values established for soil. The majority of Zn detected in the soil came from the original soil used in the column preparation and this element concentration in soil was below the reference value (60 mg kg-1). Cadmium concentration in soil was above the reference value (<0.5 mg kg-1) and it was below the intervention value (3 mg kg-1). Arsenic in soil was above the intervention value (35 mg kg-1), so that was the most critical element by the environmental point of view.
 
WARNING - Viewing this document is conditioned on your acceptance of the following terms of use:
This document is only for private use for research and teaching activities. Reproduction for commercial use is forbidden. This rights cover the whole data about this document as well as its contents. Any uses or copies of this document in whole or in part must include the author's name.
Publishing Date
2014-01-14
 
WARNING: Learn what derived works are clicking here.
All rights of the thesis/dissertation are from the authors
CeTI-SC/STI
Digital Library of Theses and Dissertations of USP. Copyright © 2001-2024. All rights reserved.